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Publication by Hanna Pazniak & Thierry Ouisse

Published on April 3, 2023
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Communique from April 2, 2023 to June 16, 2023

The article entitled "High-performance novel asymmetric MXene@CNT//N-doped CNT flexible hybrid device with large working voltage for energy storage" has been published in Journal of Energy Storage.

JESSangbegnon2023

JESSangbegnon2023

Here you will find the article by Hanna Pazniak and Thierry Ouisse:
"We developed a novel fiber-shaped supercapacitor based on a hybrid MXene@CNT//N-doped CNT device. In particular, for the first time, electrophoretically deposited Ti3C2Tx MXenes on carbon nanotube yarns and microwave-assisted nitrogen-doped carbon nanotube yarns are proposed as negative and positive electrodes, respectively. Short-circuit encountered during cell assembly was prevented entirely by coating a reproducible polyvinylidene difluoride (PVDF) membrane directly on the electrodes. Based on the developed electrodes, the assembled cell exhibited a large operating voltage window of up to 2.0 V in a diluted 0.5 M H2SO4 liquid electrolyte. The device displayed excellent stability over 5000 cycles with a Coulombic efficiency of nearly 100 %. The device withstood a floating test for 70 h with approximately 100 % capacity retention and exhibited excellent resistance to mechanical stress. Areal energy density as high as 298.5 μWh cm−2 was recorded for a power density value of 855.5 μW.cm−2 at an areal current value of 0.5 mA cm−2. At a high current density of 10 mA cm−2, the energy density remained high at 99.0 μWh cm−2 for a corresponding power density of 8.11 mW cm−2. The reported values rank among the highest obtained for carbon nanotubes-based wired-shaped supercapacitors and show the potential of this flexible wired-shaped hybrid energy storage unit as a wearable device."

 
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Date of update April 3, 2023

  • Tutelle CNRS
  • Tutelle Grenoble INP
Université Grenoble Alpes